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Imoen is the only NPC who can escape from Spellhold and reach Athkatla by herself. Any other character you abandon there is lost forever.
You can dismiss one of your party members, telling him/her to stay where he is, add Imoen and dismiss her right away, and take the other character back. This way, nobody will be pissed off. Imoen is an important part of the plot but believe me, she's not that essential and you can even finish the game without her.
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